Gösta Ekman as Faust

Emil Jannings as Mephisto

Camilla Horn as Gretchen Marguerite

Frida Richard as Gretchens's Mother

William Dieterle as Valentin

Werner Fuetterer as Erzengel

Yvette Guilbert as Marthe Schwerdtlein

Eric Barclay as Duke of Parma

Hanna Ralph as Duchess of Parma

Hans Brausewetter as Farmboy (uncredited)

Lothar Müthel as Friar (uncredited)

Hertha von Walther as (uncredited)

Hans Rameau as (uncredited)

Emmy Wyda as (uncredited)