Cliff Robertson as Cole Younger

Robert Duvall as Jesse James

Luke Askew as Jim Younger

R.G. Armstrong as Clell Miller

Dana Elcar as Allen

Donald Moffat as Manning

John Pearce as Frank James

Matt Clark as Bob Younger

Wayne Sutherlin as Charley Pitts

Robert H. Harris as Wilcox

Jack Manning as Heywood

Elisha Cook Jr. as Bunker (as Elisha Cook)

Royal Dano as Gustavson

Mary-Robin Redd as Kate

William Callaway as Calliopist

Arthur Peterson as Jefferson Jones

Craig Curtis as Chadwell

Barry Brown as Henry Wheeler

Nellie Burt as Doll Woman

Liam Dunn as Drummer

Madeleine Taylor Holmes as Granny Woman

Herbert Nelson as Chief Detective

Erik Holland as Sheriff

Anne Barton as Clell's Wife

Marjorie Durant as Maybelle

Valda Hansen as Nude Girl (as Valda J. Hansen)

Pamela Collins as Kate's Girl (uncredited)

Inger Stratton as Singing Whore