Kirk Douglas as Vincent van Gogh

Anthony Quinn as Paul Gauguin

James Donald as Theo van Gogh

Pamela Brown as Christine

Everett Sloane as Dr. Gachet

Niall MacGinnis as Roulin

Noel Purcell as Anton Mauve

Henry Daniell as Theodorus van Gogh

Madge Kennedy as Anna Cornelia van Gogh

Jill Bennett as Willemien

Lionel Jeffries as Dr. Peyron

Laurence Naismith as Dr. Bosman

Eric Pohlmann as Colbert

Jeanette Sterke as Kay

Toni Gerry as Johanna

Claire Du Brey as Housekeeper

Helen Van Tuyl as Elderly Customer

Isobel Elsom as Mrs. Stricker

David Horne as Rev. Peeters

Noel Howlett as Commissioner Van Den Berghe

William Phipps as Emile Bernard

Jay Adler as Waiter

Paul Bryar as Inspector (uncredited)

Anthony Eustrel as Tersteeg (uncredited)

Len Lesser as Cartoonist (uncredited)

George J. Lewis as Gendarme (uncredited)

Marion Ross as Sister Clothilde (uncredited)