Robert Redford as Jim Grant

Shia LaBeouf as Ben Shepard

Brendan Gleeson as Henry Osborne

Terrence Howard as FBI Agent Cornelius

Susan Sarandon as Sharon Solarz

Nick Nolte as Donal Fitzgerald

Chris Cooper as Daniel Sloan

Stanley Tucci as Ray Fuller

Julie Christie as Mimi Lurie

Richard Jenkins as Jed Lewis

Anna Kendrick as Diana

Brit Marling as Rebecca Osborne

Sam Elliott as Mac McLeod

Stephen Root as Billy Cusimano

Jackie Evancho as Isabel Grant

Keegan Connor Tracy as Jim Grant's secretary

Lochlyn Munro as FBI Agent Munro

Matthew Kimbrough as Barnes

Gabrielle Rose as Marianne Osborne

Lucie Guest as Bikini Girl

Susan Hogan as Florida Woman

Erin Simms as New York Hotel Clerk

Bethany Brown as Record Store Clerk

Kelly-Ruth Mercier as Gas Station Cashier

Gabriela Reynoso as Maria

Marsha Regis as Albany Times Assistant

Andrea Brooks as Sharon Solarz's Daughter

Dawn Chubai as News Anchorwoman #1

Sophie Lui as News Anchorwoman #2

Allison Riley as New York Newswoman

Donna Lysell as Eva Sloan

Nicole G. Leier as Gas Station Customer

Jennifer Bradley as Billy Cusimano's Daughter

David Milchard as Ann Arbor County Clerk

David James Lewis as Albany FBI Agent Lewis

Jon Johnson as Albany FBI Agent Johnson

Isaiah Adam as New York Cameraman

John Shaw as DMV Source

Bernie Yao as Car Rental Clerk

Bruce Dawson as Sharon Solarz's Husband

Jackson Warris as Sharon Solarz's Son

Dale Wolfe as Ann Arbor Reporter

Mark Brandon as New York Anchor #1

Jan Bos as New York Anchor #2

Clay St. Thomas as 80's Reporter

Barry Bowman as 80's Newsman

Fred Henderson as 80's Anchorman

Dan Gerrity as 70's News Anchor

Mark Pawson as On-Site Journalist

Jason Blue as Rebecca's Date

Peter Jenkins as Dad on Train

G. Michael Gray as Drunk on Train

Ed Huber as Daniel Sloan's Doorman

Ian Gregson as Hotel Guest (uncredited)

Pierre Wolff as Ben's Father (uncredited)

Anthony Welch as Drug Smuggler (uncredited)

Jessica Williams as Jess (uncredited)

Lexie Huber as Jim's Wife (uncredited)

Nicole Smashnuk as Woman who lost shoe in evacuation (uncredited)