Laurence Harvey as Wilhelm Grimm / Cobbler (segment "The Cobbler and the Elves")

Karlheinz Böhm as Jacob Grimm

Claire Bloom as Dorothea Grimm

Walter Slezak as Stossel

Barbara Eden as Greta Heinrich

Oskar Homolka as The Duke ('The Dream')

Arnold Stang as Rumpelstiltskin

Martita Hunt as Anna Richter

Betty Garde as Miss Bettenhausen

Bryan Russell as Friedrich Grimm

Ian Wolfe as Gruber

Tammy Marihugh as Pauline Grimm

Cheerio Meredith as Mrs. Von Dittersdorf

Walter Rilla as Priest

Yvette Mimieux as The Princess (segment "The Dancing Princess")

Russ Tamblyn as The Woodsman (segment "The Dancing Princess") / Tom Thumb

Jim Backus as The King (segment "The Dancing Princess")

Beulah Bondi as The Gypsy (segment "The Dancing Princess")

Clinton Sundberg as The Prime Minister / Hans (singing voice)

Walter Brooke as The Mayor (segment "The Cobbler and the Elves")

Sandra Bettin as The Ballerina (segment "The Cobbler and the Elves")

Robert Foulk as The Hunter (segment "The Cobbler and the Elves")

Terry-Thomas as Ludwig (segment "The Singing Bone")

Buddy Hackett as Hans (segment "The Singing Bone")

Otto Kruger as The King (segment "The Singing Bone")

Robert Crawford Jr. as The Shepherd (segment "The Singing Bone")

Sydney Smith as The Spokesman (segment "The Singing Bone")

Pamela Baird as Cinderella (uncredited)

Billy Barty as The Court Jester (segment "The Dancing Princess") (uncredited)

Jeanine Cashell as Princess Aide ('The Dancing Princess') (uncredited)

Diana Driscoll as Gretel

True Ellison as Snow White

Stanley Fafara as Hansel

Darby Hinton as Little Boy

Jon Lormer as The Doctor

Gregory Morton as Dantino

Elisabeth Neumann-Viertel as Flower Vendor

'Little Billy' Rhodes as Grumpy the Dwarf

Ruthie Robinson as Little Red Riding Hood

Angelo Rossitto as Dwarf

Gene Roth as Berlin Royal Academy Representative at Train Station

Peter Whitney as The Giant