Sean Connery as James Bond

Daniela Bianchi as Tatiana 'Tanja' Romanova

Pedro Armendáriz as Ali Kerim Bey

Robert Shaw as Donald 'Red' Grant

Lotte Lenya as Rosa Klebb

Bernard Lee as M

Lois Maxwell as Miss Moneypenny

Eunice Gayson as Sylvia Trench

Walter Gotell as Morzeny

Francis de Wolff as Vavra

George Pastell as Train Conductor

Nadja Regin as Kerim's Mistress

Aliza Gur as Vida

Martine Beswick as Zora

Vladek Sheybal as Kronsteen

Anthony Dawson as Ernst Stavros Blofeld

Lisa Guiraut as Belly Dancer

Hasan Ceylan as Bulgarian Agent

Fred Haggerty as Krilencu

Neville Jason as Kerim's Chauffeur

Peter Bayliss as Benz

Nusret Ataer as Mehmet

Peter Brayham as Rhoda

Desmond Llewelyn as Boothroyd - 'Q'

Jan Williams as Masseuse

Peter Madden as McAdams

Fred Wood as Gypsy (uncredited)

Bill Brandon as Gypsy (uncredited)

Moris Farhi as Gypsy (uncredited)

Alf Mangan as Gypsy (uncredited)

Dido Plumb as Gypsy (uncredited)

Ernie Rice as Gypsy (uncredited)

Andre Charisse as Hotel Concierge (uncredited)

Hugo de Vernier as Hotel Porter (uncredited)

Victor Harrington as Chess Tournament Spectator (uncredited)

Barbara Jefford as Tatiana Romanova (voice) (uncredited)

Jim Brady as Krilencu's Henchman (uncredited)

Eric Pohlmann as Ernst Stavro Blofeld (voice) (uncredited)

Bob Simmons as James Bond in Gunbarrel Sequence (uncredited)

Nikki Van der Zyl as Sylvia Trench / Receptionist (voice) (uncredited)

Michael Culver as Man in a Punt (uncredited)

Elizabeth Counsell as Woman in a Punt (uncredited)

Bedri Çavusoglu as Police (uncredited)