Finn Atkins as Charlotte Brontë

Chloe Pirrie as Emily Brontë

Charlie Murphy as Anne Brontë

Adam Nagaitis as Branwell Brontë

Jonathan Pryce as Patrick Brontë

Luke Newberry as George Smith

Rebecca Callard as Miss Pratchett

James Norton as Duke of Wellington

Jill Baker as Aunt Branwell

Rory Fleck-Byrne as Arthur Nicholls

David Walmsley as Joseph Bentley Leyland

June Watson as Tabby

Thomas Nelstrop as Dr. Wheelhouse

Joe Armstrong as Thomas Mallinson

David Prosho as Bailiff - Mr Riley

Gracie Kelly as Ellen Nussey

Rosie Boore as Young Charlotte Brontë

Thomas Howes as Samuel Hartley

Hugh Simon as William Smith Williams

Megan Parkinson as Martha Brown

Mark Frost as John Brown

Paul Kynman as Henchman

Nigel Black as High Flyer

Troy Tipple as Young Branwell Brontë

Kris Mochrie as Captain John

Jamie Dorrington as Enoch Thomas

Freddie Meredith as Kent

Lara McDonnell as Young Anne Brontë

Jonathon Carley as Napoleon Bonaparte

Karen Shaw as Mrs. Robinson

Talia Barnett as Young Emily Brontë

Matt Adams as Captain Parry / Jack Sharp

John Ammirati as Londoner