Melissa Altro as Pippi Longstocking (voice)

Catherine O'Hara as Mrs. Helga Prysselius (voice)

Gordon Pinsent as Capt. Efraim Longstocking (voice)

Dave Thomas as Thunder-Karlsson (voice)

Wayne Robson as Bloom (voice)

Noah Reid as Tommy Settegren (voice)

Olivia Garratt as Annika Settegren (voice)

Judy Tate as Annika Settegren (singing voice)

Carole Pope as Teacher (voice)

Karen Bernstein as Mrs. Ingrid Settegren (voice)

Martin Lavut as Mr. Sven Settegren (voice)

Rick Jones as Constable Kling / O'Malley (voice)

Philip Williams as Constable Klang / Ringmaster (voice)

Mari Trainor as Mrs. Kling (voice)

Elva Mai Hoover as Mrs. Klang (voice)